Michael Portillo did an investigation of methods of capital punishment, and concluded that all current methods were inhumane in one way or another, either to the condemned or to the executioner. One way, not currently used, seemed to fit all the criteria though: oxygen deprivation through replacement with inert gases. It was amusing to watch him squirming at the results of each test, or in some cases putting himself through the paces (through a lower non-lethal dosage, of course). In the last case, oxygen deprivation, he became more and more incoherent until he zoned out and the observer ended the experiment.
Portillo Seconds From Death - Horizon:How to Kill a Human...
Said documentary directly prompted Oklahoma to change its method of implementing the death penalty. AFAIK no executions have yet been done using the new method.
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